Equilibrium and Kinetic Study of Reactive Dye Brilliant Red HE-3B Adsorption by Activated Charcoal
Daniela Suteu* and Doina Bilba
Department of
Analytical Chemistry, “Gh.Asachi”, Technical University of Iasi, Bl. D.
Mangeron, 71A Iassi, 700050, Romania
E-mail: dsuteu@ch.tuiasi.ro;
danasuteu@go.ro
Abstract
The commercially
powdered activated charcoal was used for the sorption of reactive dye Brilliant
Red HE-3B from aqueous solutions. The effect of solution pH, initial dye
concentration, temperature and sorption time on dye removal was studied. The
equilibrium sorption isotherms have been analysed by the linear, Freundlich and
Langmuir models. The Langmuir isotherms have the highest correlation
coefficients. The apparent thermodynamic parameters were calculated and the
obtained values support the conclusion that the reactive dye molecules sorbs by
entropy-driven, endothermic process. The kinetic of the sorption was analysed
using the pseudo-first order and pseudo-second order kinetic models. The data
showed that the second-order equation was the more appropriate, which indicate
that the intraparticle diffusion is the rate limiting factor.
Key words: sorption, activated charcoal, reactive dye, equilibrium, kinetic